Chapter 7: Carboxylic Acids

B.Sc. 2nd Year Chemistry – Detailed and Exam-Oriented Notes

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1. Introduction

Carboxylic acids are an important class of organic compounds containing the carboxyl functional group, –COOH. The carboxyl group consists of a carbonyl group (>C=O) and a hydroxyl group (–OH) attached to the same carbon atom.

General structure: R–COOH

Carboxylic acids are widely distributed in nature. Examples include formic acid in ants, acetic acid in vinegar, benzoic acid in some natural products and fatty acids in fats and oils.

The acidic character of these compounds is mainly due to the ability of the carboxyl group to lose a proton and form a resonance-stabilized carboxylate ion.

Key concept: Resonance stabilization of the carboxylate ion is the major reason why carboxylic acids are more acidic than alcohols.

2. Structure of the Carboxyl Group

The carboxyl group contains two important functional components: a carbonyl group and a hydroxyl group.

R–C(=O)–OH

The carbon atom of the carboxyl group is approximately sp2-hybridized. The group is approximately planar because of conjugation between the carbonyl system and the hydroxyl oxygen.

When a carboxylic acid loses a proton, the resulting carboxylate ion is stabilized by resonance.

R–COO ↔ R–C(O)=O

The negative charge is delocalized over the two oxygen atoms, making the carboxylate ion considerably more stable than a localized alkoxide ion.

3. Classification of Carboxylic Acids

3.1 Monocarboxylic Acids

Compounds containing one carboxyl group are called monocarboxylic acids.

Examples: Methanoic acid and ethanoic acid.

3.2 Dicarboxylic Acids

Compounds containing two carboxyl groups are called dicarboxylic acids.

Examples: Oxalic acid and malonic acid.

3.3 Polycarboxylic Acids

Compounds containing more than two carboxyl groups are called polycarboxylic acids.

3.4 Aliphatic Carboxylic Acids

The carboxyl group is attached to an aliphatic carbon chain.

Example: CH3COOH.

3.5 Aromatic Carboxylic Acids

The carboxyl group is directly attached to an aromatic ring.

Example: Benzoic acid, C6H5COOH.

4. Nomenclature of Carboxylic Acids

In IUPAC nomenclature, the longest carbon chain containing the carboxyl carbon is selected and the suffix -oic acid is used.

Common name IUPAC name Formula
Formic acid Methanoic acid HCOOH
Acetic acid Ethanoic acid CH3COOH
Propionic acid Propanoic acid CH3CH2COOH
Butyric acid Butanoic acid CH3CH2CH2COOH
Benzoic acid Benzoic acid C6H5COOH

The carbon atom of the carboxyl group is assigned position 1 when numbering the parent chain.

5. Preparation of Carboxylic Acids

5.1 Oxidation of Primary Alcohols

Primary alcohols can be oxidized first to aldehydes and then further to carboxylic acids using suitable oxidizing agents.

RCH2OH + 2[O] → RCOOH + H2O

5.2 Oxidation of Aldehydes

Aldehydes are readily oxidized to corresponding carboxylic acids.

RCHO + [O] → RCOOH

5.3 Hydrolysis of Nitriles

Nitriles can be hydrolyzed under acidic or alkaline conditions to produce carboxylic acids or their salts, followed by acidification.

R–CN + 2H2O → R–COOH + NH3

5.4 Hydrolysis of Esters

Esters undergo hydrolysis to give a carboxylic acid and an alcohol under acidic conditions.

RCOOR′ + H2O ⇌ RCOOH + R′OH

5.5 Hydrolysis of Amides

Amides can undergo hydrolysis under suitable acidic or basic conditions to give carboxylic acids or carboxylate salts.

5.6 Grignard Reagent and Carbon Dioxide

Grignard reagents react with carbon dioxide to form magnesium carboxylates, which give carboxylic acids on hydrolysis.

RMgX + CO2 → RCOOMgX
RCOOMgX + H3O+ → RCOOH + Mg salts

6. Physical Properties

Carboxylic acids show strong intermolecular association because they can form hydrogen bonds.

Dimer Formation

Carboxylic acids commonly form hydrogen-bonded dimers, especially in non-polar solvents and vapor phase.

2RCOOH ⇌ (RCOOH)2

The formation of dimers contributes to their relatively high boiling points.

7. Acidic Nature of Carboxylic Acids

Carboxylic acids are weak acids but are considerably stronger acids than alcohols and many simple hydrocarbons.

RCOOH ⇌ RCOO + H+

Their acidic strength is explained by the stability of the conjugate base, the carboxylate ion.

Resonance Stabilization

The negative charge of the carboxylate ion is delocalized over the two oxygen atoms.

R–COO ↔ R–C(O)=O

Because the negative charge is distributed over two electronegative oxygen atoms, the carboxylate ion is stabilized.

Comparison with Alcohols

Alkoxide ions formed from alcohols do not have equivalent resonance stabilization. Therefore, alcohols are generally much weaker acids than carboxylic acids.

8. Effect of Substituents on Acidity

The acidity of a carboxylic acid is affected by electron-withdrawing and electron-donating groups attached to the carbon chain.

8.1 Electron-Withdrawing Groups

Electron-withdrawing groups such as halogens generally increase acidity by stabilizing the negative charge of the carboxylate ion through the inductive effect.

8.2 Electron-Donating Groups

Alkyl groups generally show an electron-donating inductive effect and tend to decrease acidity relative to the parent acid.

General rule: Electron-withdrawing groups near the carboxyl group generally increase acidity, while electron-donating groups generally decrease acidity.

9. Reaction with Active Metals

Carboxylic acids react with active metals such as sodium to form carboxylate salts with liberation of hydrogen gas.

2RCOOH + 2Na → 2RCOONa + H2

Evolution of hydrogen gas provides evidence of the acidic nature of carboxylic acids.

10. Reaction with Bases

Carboxylic acids react with sodium hydroxide and other strong bases to form salts and water.

RCOOH + NaOH → RCOONa + H2O

This is a neutralization reaction.

11. Reaction with Carbonates and Bicarbonates

Carboxylic acids react with sodium carbonate or sodium bicarbonate to produce carbon dioxide gas.

With Sodium Bicarbonate

RCOOH + NaHCO3 → RCOONa + CO2↑ + H2O

With Sodium Carbonate

2RCOOH + Na2CO3 → 2RCOONa + CO2↑ + H2O
Laboratory identification: Effervescence due to carbon dioxide evolution is a characteristic test for carboxylic acids.

12. Esterification

Carboxylic acids react with alcohols in the presence of a strong acid catalyst, commonly concentrated sulfuric acid, to form esters.

RCOOH + R′OH ⇌ RCOOR′ + H2O

This reaction is called Fischer esterification. The reaction is reversible and is often driven toward ester formation by removing water or using an excess of one reactant.

Many esters have pleasant fruity or floral odors and are important in flavor and fragrance chemistry.

13. Formation of Acid Chlorides

Carboxylic acids react with chlorinating agents such as thionyl chloride to form acid chlorides.

RCOOH + SOCl2 → RCOCl + SO2 + HCl

Acid chlorides are highly reactive carboxylic acid derivatives and are useful intermediates in organic synthesis.

14. Formation of Amides

Carboxylic acids can form amides through reactions involving ammonia or amines under appropriate conditions.

Initially, an ammonium carboxylate may be formed. Heating can promote dehydration to give an amide.

RCOOH + NH3 → RCOONH4+
RCOONH4+ → RCONH2 + H2O

15. Reduction of Carboxylic Acids

Carboxylic acids can be reduced to primary alcohols using strong reducing agents such as lithium aluminium hydride.

RCOOH + 4[H] → RCH2OH + H2O

Reduction of the carboxyl group to an alcohol is an important transformation in organic synthesis.

16. Decarboxylation

Decarboxylation is the removal of carbon dioxide from a carboxylic acid or its salt.

Soda Lime Decarboxylation

Sodium salts of carboxylic acids undergo decarboxylation when heated with soda lime, producing an alkane containing one carbon atom fewer than the original acid.

RCOONa + NaOH → RH + Na2CO3

Soda lime is generally a mixture of sodium hydroxide and calcium oxide.

Example

CH3COONa + NaOH → CH4 + Na2CO3

17. Hell-Volhard-Zelinsky Reaction

Carboxylic acids containing an alpha-hydrogen can undergo alpha-halogenation in the presence of halogen and phosphorus-based reagents.

The reaction introduces a halogen atom at the alpha carbon of the carboxylic acid.

RCH2COOH → RCHXCOOH

The reaction is useful for preparing alpha-halo carboxylic acids, which are valuable intermediates in organic synthesis.

18. Derivatives of Carboxylic Acids

Important derivatives of carboxylic acids are compounds in which the hydroxyl group of the carboxyl group is replaced by another group.

Derivative General formula Example
Acid chloride RCOCl CH3COCl
Acid anhydride (RCO)2O (CH3CO)2O
Ester RCOOR′ CH3COOCH3
Amide RCONH2 CH3CONH2

19. Relative Reactivity of Acid Derivatives

Carboxylic acid derivatives differ in their reactivity toward nucleophilic acyl substitution.

Acid chloride > Acid anhydride > Ester ≈ Acid > Amide

Acid chlorides are highly reactive because chloride ion is a good leaving group and the carbonyl carbon remains strongly electrophilic. Amides are comparatively less reactive because the nitrogen lone pair participates in resonance with the carbonyl group.

20. Important Carboxylic Acids

20.1 Formic Acid

Formic acid, HCOOH, is the simplest carboxylic acid. It occurs naturally in the venom of ants and certain other organisms.

It is a colorless liquid with a pungent odor and has applications in leather processing, textiles and preservation.

21. Acetic Acid

Acetic acid, CH3COOH, is an important industrial and biological carboxylic acid. Dilute aqueous acetic acid is the principal acid present in vinegar.

Pure acetic acid freezes near room temperature and is therefore commonly referred to as glacial acetic acid when highly concentrated.

Important Uses

22. Oxalic Acid

Oxalic acid is a dicarboxylic acid with the formula HOOC–COOH.

It occurs naturally in some plants and can form insoluble salts with certain metal ions.

Oxalic acid and oxalates are also important in analytical chemistry and laboratory applications.

23. Benzoic Acid

Benzoic acid, C6H5COOH, is the simplest aromatic carboxylic acid.

It is a crystalline solid and has important applications in food preservation and organic synthesis.

Reaction with Sodium Hydroxide

C6H5COOH + NaOH → C6H5COONa + H2O

24. Important Dicarboxylic Acids

Acid Structure
Oxalic acid HOOC–COOH
Malonic acid HOOC–CH2–COOH
Succinic acid HOOC–CH2–CH2–COOH
Glutaric acid HOOC–(CH2)3–COOH
Adipic acid HOOC–(CH2)4–COOH

Several dicarboxylic acids are important intermediates in polymer production and biochemical pathways.

25. Comparison of Carboxylic Acids and Alcohols

Property Carboxylic acids Alcohols
Functional group –COOH –OH
Acidity Higher Much lower
Conjugate base Resonance-stabilized carboxylate ion Alkoxide ion
Reaction with NaHCO3 CO2 evolved Generally no reaction
Typical reaction Esterification Oxidation, substitution, dehydration

26. Important Reactions for Revision

RCOOH + NaOH → RCOONa + H2O
RCOOH + NaHCO3 → RCOONa + CO2 + H2O
RCOOH + R′OH ⇌ RCOOR′ + H2O
RCOOH + SOCl2 → RCOCl + SO2 + HCl
RCOOH + 4[H] → RCH2OH + H2O
RCOONa + NaOH → RH + Na2CO3
RMgX + CO2 → RCOOMgX → RCOOH
RCHO + [O] → RCOOH

27. Applications and Importance

28. Biological Importance

Carboxylic acids are widely distributed in biological systems.

29. Important Points for Examination

30. Chapter Summary

Carboxylic acids contain the –COOH functional group and are among the most important oxygen-containing organic compounds.

Their acidic nature results from the resonance stabilization of the carboxylate ion formed after loss of a proton.

They can be prepared by oxidation of primary alcohols and aldehydes, hydrolysis of nitriles, esters and amides, and reaction of Grignard reagents with carbon dioxide.

Important reactions include neutralization, reaction with metals, reaction with carbonates, esterification, formation of acid chlorides and amides, reduction and decarboxylation.

Important reactions for examination include Fischer esterification, soda-lime decarboxylation and the Hell-Volhard-Zelinsky reaction.

Carboxylic acids and their derivatives have extensive applications in food chemistry, pharmaceuticals, polymers, biological systems and industrial organic synthesis.

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